Structure and Properties of dmit Systems
	構造	伝導度	その他	
Ni(dmit)2	P21/a (#43)			
TTF[Ni(dmit)2]2	C2/c (#30)
バンド構造
（#34およびR1）	σrt =300 (#30)
Tc=1.6K (7kbar) (R3,#33等)
常圧下では金属	χ(#4), NMR(#28)
温度－圧力相図(#33)
物性一般（R3の文献を見よ）	
α-EDT-TTF[Ni(dmit)2]	P1-(#7, #22)
交差型	σrt =100(//ab) (#7)
σrt =140~370(//ab);
σrt =14~36(//c*) (#14)
TM-M=14 K(#7)
TSC=1.3K(#8)	Magnetoresistance(#9)
Hc2 (#10)
Opt. (#11)
Meissner (#12）
χ (#13)
ESR (#22)	
β-EDT-TTF[Ni(dmit)2]	mixed stack
P21/c (#7)	σrt =0.01; semicon.		
γ-EDT-TTF[Ni(dmit)2]	1D (#22)	σrt =100; TM-I=100 K		
TMTSF[Ni(dmit)2]	1D (TMTSF)
(#19)	σrt =300 ;semicon. Ea=0.034eV (#19)		
α-(BPDT-TTF) [Ni(dmit)2]2	1D (#20)	σrt =5~10; Ea= 0.012eV (r.t.~120K) ; TS-S=120 K (#20)		
(DBTTF)[Ni(dmit)2]	2-chain
(#23)	σrt =100		
(ET)[Ni(dmit)2]	mixed stack (#24)	σrt =10-3
;Ea=0.28eV		
OMTSF[Ni(dmit)2] (#50)	mixed stack (#50)	σrt =10(#50)	Opt(#50)	
[Pt(dddt)2[Ni(dmit)2]	monoclinic
(#53)	insulator		
(NH2Me2)[Ni(dmit)2]2	P1-(#6,#48)	σrt =0.08(//ab) (#6)
semicon. Ea=0.2eV		
(NHMe3)[Ni(dmit)2]2	P1-(#48)	σrt =140; semicon.		
(NHMe3)2[Ni(dmit)2]5. 2CH3CN	P1-(#48)	σrt =0.2(//ab) (#6)
semicon. Ea=0.2eV		
(NH3Me)2[Ni(dmit)2]5. 2CH3CN	P1-(#48)	σrt =1.5(//ab) (#6)
semicon. Ea=0.2eV		
α-Et2Me2N[Ni(dmit)2]2	C2/c(R.T.;#16)
P21/c(17K:#27)
2DFS(#27)	σrt =20~100(//bc) (#16); σrt =2.5(//a*) (#17)
TM-M=245 K (#17)	SdH (#17,#18)
AMRO (#17)
χ(#54)	
γ-Et2Me2N[Ni(dmit)2]2	Pnma (RT); P212121(4.3K) ; (#54)	metallic 
metal-metal transitionをしめさない(#54)	χ(#54)	
(C7H16N)[Ni(dmit)2]2	C2/c (300K)
Cc(20K) (#51)	metallic down to 0.5K (#51)  TM-M=225K	χ(#54)	
(Et4N)0.5[Ni(dmit)2]	(#25)	σrt(//b) =4.510-2; semicon. (#25)		
(CH3)4N[Ni(dmit)2]2	C2/c (#39)
X-ray 温度依存性(#39)
FS (#39a,c, #32) 	σrt =50(#32); TM-I =40K, TI-I=20 K(#41); Tsc=5K(7kbar;#39)	χ(#41), S(#41), Opt.(#42a)	
[Bu4N]2[Ni(dmit)2]7. 2CH3CN	P1- (#43)	σrt =1-10; semicon.; Ea=0.1~0.02eV (#43)	Opt.(#52)	
(Ph4As)0.25[Ni(dmit)2]	P2/n(#45)	σrt =10-15;  semicon.; Ea=0.03~0.01eV (#45)		
Ph4P[Ni(dmit)2]3	C2/c 
(#52)	σrt =10;Ea~46meV
semicon. (#36)
σrt =7; semicon; Ea = 0.01eV (#52)	χ, opt, S  (#36)
Opt.(#52)	
Me(Ph)3P[Ni(dmit)2]3
	P21/c (#56)	0.07~0.1; Ea=0.22eV
(#56)		
(Me3S)[Ni(dmit)2]2	P1- (#52)	σrt =6.510-2; semicon.; Ea=0.13eV (#52)	Opt.(#52)	
AcrH[Ni(dmit)2]3	C2/c (#75, #76)	σrt =45
metallic down to 4K		
MEA[Ni(dmit)2]3. MeCN	P21/c (#74)			
Hmorph2[Ni(dmit)2]3	P21/n (#74)	σrt =0.1; semicon.; Ea=0.1eV		
HMemorph[Ni(dmit)2]2	P1- (#74)	σrt =4; semicon.; Ea=0.1eV		
[guanidinium] [Ni(dmit)2]2	P1- (#63)	σrt =32; semicon.; Ea=0.12eV (#63)		
[1,1-dimethylguani-dinium][Ni(dmit)2]2	P1- (#63)	σrt =0.15; semicon.; Ea=0.13eV (#63)		
[Me3N(CH2)4NMe3] [Ni(dmit)2]5.2dmf	P1-(#64)	σrt =1; semicon.; Ea=0.0.19eV (#64)		
[Me3N(CH2)4NMe3] [Ni(dmit)2]5.2CH3CN	P1(#64)	σrt =0.1; semicon.; Ea=0.20eV (#64)		
[Li]2[12-crown-4]3. [Ni(dmit)2]7[acetone]2	P1-(#58,#59)	σrt =30; semicon.; Ea=0.1 eV(T>230K), Ea=0.17eV (T<230K) (#58,#59)		
[NH4][15-crown-5]2. [Ni(dmit)2]	C2/c(#58)	σrt =10-6; insulator (#58)		
[NH4][18-crown-6]. [Ni(dmit)2]3	P1-(#58)	σrt =0.4; semicon.; Ea=0.15 (T>230K), Ea=0.07eV (T<230K) (#58)		
Li0.6(15-crown-5-ether)[Ni(dmit)2]2.H2O	P21/c (#60)	σrt =240; TM-I=250 K (#60)	χ, NMR(#60)	
Li[Ni(dmit)2]2.2CH3CN
(1); Na[Ni(dmit)2]2 (2); K0.4[Ni(dmit)2] (3); Rb0.36[Ni(dmit)2] (4); Cs[Ni(dmit)2]2 (5) 		(1) σrt =0.5;semicon.
(2) σrt =20;metal
(3) σrt =100;metal
(4) σrt =10;semicon.
(R3)		
p-EYPNN[Ni(dmit)2]	P1-
spin-ladder(#38)	σrt =1.310-4(#38); Semicon.	χ(#38)	
C1+[Ni(dmit)2]- (1)
C1+[Ni(dmit)2]- (2)
C2+[Ni(dmit)2]- (3)
C2+[Ni(dmit)2]- (4)
C1,C2=Cyanine Dyes	(1),(3) P21/c
(2),(4) P1-

(#55)	σrt[(2)~(3)] =10-6~10-5 (powder)
σrt[(1)] =1.310-2
Ea=0.05eV (#55)		
				
(α,α')-TTF[Pd(dmit)2]2
（二つの相が同じ物か別かが不明 ）
	C2/c (#29;R3)
TTF[Ni(dmit)2]2と同型構造
E(k) (#34: α')	σrt =750 (α,α'共:R3)
TM-I=220K(1 bar)
Tsc=5.9K(24kbar: α')
Tsc=1.2K(19.25kbar: α)  (#35)	χ(#4: α' ,αの区別なし)	
β-TTF[Pd(dmit)2]2	P1-(#29)			
γ-TTF[Pd(dmit)2]2	P1-(#29)			
γ-TTF[Pd(dmit)2]2	P1-(#29)	100 TM-I=100 (#29)		
α'-EDT-TTF[Pd(dmit)2]	P1- (#47)
Fermi面(#47, #31)	σrt =58
TM-M=40K 
metal  (#31)	X-Ray; χ (#47)	
EDT-TTF2[Pd(dmit)2]3	P1-; E(k) (#47)	σrt =120; (#47) 温度依存性のデータなし		
γ-EDT-TTF[Pd(dmit)2]	diffuse,温度依存性を含む(#22)	σrt(//:2.4kbar)~150; TM-M=80K(#22); metallic down to 2K (2.4kbar) (#22)		
IEDT[Pd(dmit)2]	P1-(#67)	σrt =300; metallic down to 4.2K (#67)		
Cs[Pd(dmit)2]2	C2/c (#15;#34)	σrt =100(//ab) (#15)	σ,χ,Opt.(#15;#42)	
Et2Me2N[Pd(dmit)2]2	P1-
open FS (#57)	σrt =10~80; Tsc = 4K (2.4kbar)  (#57)		
α-(CH3)4N[Pd(dmit)2]2	P1- (#26)	σrt =50; semicon.(1bar)		
β-(CH3)4N[Pd(dmit)2]2	C2/c(#26) ;FS (#70,#71, #72)
	σrt =30; semicon.(1bar)
Tsc=6.2K(6.5 kbar) (#70）		
β-(CH3)4As[Pd(dmit)2]2	C2/c (#26); FS(#71, #72)	σrt =1; semicon.; Ea = 0.07 eV; 高圧下で4.2Kまで金属的(#72)	Opt. (#42)	
β-(CH3)4P[Pd(dmit)2]2	C2/c (#37); FS (#71, #72)
	σrt =20; TM-I=60 K; σrt =1; semicon.; Ea=0.07 eV (#37); 高圧下で4.2Kまで金属的(#72)	χ(#72)	
β-(CH3)4Sb[Pd(dmit)2]2	C2/c ;FS (#71, #72)	σrt =20; semicon.; 高圧下で4.2Kまで金属的 (#71, #72)		
(Et4N)0.5[Pd(dmit)2]	(#62,R3)	σrt =0.11; semicon.(R3)		
n-Bu4N0.5[Pd(dmit)2]	P1-(#61)	σrt =12; TM-I=240 K (#61)		
(n-Bu4N)0.33[Pd(dmit)2]	P1-(#61)	σrt =150; TM-I=120K (initial); semicon. (after heat cycle) (#61)		
β'-Et2Me2P[Pd(dmit)2]2	C2/c (#69)	σrt =10; semicon.; 
Tsc=4 K at 6.9 kbar
(#68)	特異な相図
χ	
β'-Et2Me2Sb[Pd(dmit)2]2	C2/c (#69)	σrt =1; semicon.; 
高圧下で金属的 (#68)		
				
TTF[Pt(dmit)2]3	P1-(#30)	σrt =20; Ea=0.03eV (300-200K: #30)		
(HMTTeF)2[Pt(dmit)2]	2D (#21)	σrt =5~10; semicon.;		
CH3N[Pt(dmit)2]2	C2/c(#1)
Band Structure (#1)	σrt =10(//ab) (#1)
TMI = 220 K	Opt. (#2)	
(NHMe3)[Pt(dmit)2]3. CH3CN	P1-(#5,#48)	σrt =140(//ab) (#5; #6)
TMI = 180 K		
				
Me4N[Au(dmit)2]2	B2/b(#3)	σrt =5-15(//a) (#3)
Semicon.		
Et4N[Au(dmit)2TCNQ]	P1-(#49)	σrt =110-5(#49)	opt. (#49)	
				
(ET)3[V(dmit)3]2	P1-(#46a)
E(k) (#46b)	σrt =3-45; semicon. ;Ea=0.020eV T<150 K		
[NBu4]2[W(dmit)3]	Pca21(#44)	insulator		
[NBu4]2[Mo(dmit)3]	Pca21(#44)	insulator		
[Fe(C5Me5)2][W(dmit)3]	P1-(#44)	insulator	χ	
				
α-[Me4N][Ni(dmise)2]2	Pbnb (#65)
	σrt =1; semicon.; Ea=0.08eV (#65)		
β-[Me4N][Ni(dmise)2]2	C2/c (#65)	σrt =10; semicon.; Ea=0.05eV  (#65)		
D [Pd(dmise)2]2 
(1): D=(CH3)4N;
(2): D=(CH3)4P;
(3): D=(CH3)4As;
(4): D=(CH3)4Sb;	C2/c; E(k)
(#66, #72)	σrt =200~20; 
TM-I=150 K
(#66); 圧力依存性を含めた詳細なデータ(#72)	(2):χ (#72); NMR(#73)	
				
NMe4[Pd(dsit)2]2	C2/c (#37)	σrt =30-70 (#37)
TM-I=220K	Opt (#37)	

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(#67)T. Imakubo, H. Sawa, R. Kato, J. Chem. Soc., Chem., Commun., 1995, 1097.
(#68)R. Kato, Y. Kashimura, S. Aonuma, N. Hanasaki, H. Tajima, Solid State Commn., 105, 561(1998).
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(#71)R. Kato, Y.-L. Liu, S. Aonuma, H. Sawa, Solid State Commn., 98, 1021(1996).
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(#73)T. Tsuchiya, T. Nakamura, T. Takahashi, Y.-L. Liu, H. Sawa, R. Kato, Synthetic Metals, 86, 2117(1997). 
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(#75)Y. S. J. Veldhuizen, J. G. Haasnoot, J. Reedijk, Synth. Met., 86, 1827(1997).
(#76) Y. S. J. Veldhuizen, W. J. J. Smeets, N. Veldman, A. L. Spek, C. Faulmann, P. Auban-Senzier, D. Jerome, P. M. Paulus, J. G. Haasnoot, J. Reedijk, Inorg. Chem., 36, 4930(1997).

増補
1) "M(dmit)2 salts with Nitronyl nitroxide radical cations (M=Ni and Au, dmit=1,3-Dithiol-2-thione-4,5-dithiolate). Nonmagnetic single-chain formation vs Antiferromagnetic Spin-Ladder-chain formation of M(dmit)2"
H. Imai, T. Otsuka, T. Naito, K. Awaga, and T. Inabe, J. Am. Chem. Soc., 121, 8098-8103(1999).
2)"Upper critical field of the molecular superconductor b'-ET2Me2P[Pd(dmit)2]2"
S. Rouziere, N.Hanasaki, R. Kato, and H. Tajima, Solid State Commun., 112, 295-300(1999).
3)"Low-temperature structural studies of molecular b'-Pd(dmit)2 conductors"
S. Rouziere, J.-I.Yamaura, and R. Kato, Phys. Rev. B, 60, 3113-3119(1999).
4)"Preparation, structure and properties of [Na(cis-antt-cis-dicyclohexyl-18-crown-6)][Ni(dmit)2)]4.2Me2CO"
N. Robertson. T. Akutagawa,T. Nakamura, S. Roehrs, and A. E. Underhill, J. Mater. Chem., 9, 1233-1236(1999).
5)"Dramatic anion size effect on structural and magnetic propertiswithin a series of novel antiferromagnetic organometallic radical cation salts:[Cp2Mo(dmit)+.][X-] (X-=PF6-, AsF6-, SbF6-)
R.Clerac,M.Fourmigue, J.Gaultier, Y. Barrans, and P.A. Albouy, Eur. Phys. J. B, 9, 431-443.
6)"Experimental determination and modelization of a unique phase diagram: solid solutions of antiferromagnetic organometallic radical cation salts [Cp2Mo(dmit)+.] [X-](x) [PF6-](1-x) (X-= AsF6-, SbF6-)"
R.Clerac,M.Fourmigue, J.Gaultier, Y. Barrans, and P.A. Albouy, Eur. Phys. J. B, 9, 445-459.
7)"First-principles study of the electronic structure of the organic solids (CH3)4N[M(dmit)2]2 (M=Ni and Pd): Role of dimerization and stability of the formation of a dimer"
T. Miyazaki and T. Ohno, Phys. Rev. B, 59, 5269-5272 (1999).
8)"Synthesis, Structure, and Physical Properties of Tetraalkylammonium Bis(5,6-dihydro-1,4-dithiin-2,3-diselenolato)nickelate, (R4N)[Ni(ddds)2] (R=Me,Et,and n-Bu), and natural complex [Ni(ddds)2]2"
H. Fujiwara, E. Ojima, H. Kobayashi, T. Courcet, I. Malfant, and P. Cassoux, Eur. J. Inorg. Chem., 1998, 1631-1639.